秦山核电基地大气多形态氚的分布

doi:10.11889/j.0253-3219.2019.hjs.42.070601

Nuclear Techniques ›› 2019, Vol. 42 ›› Issue (7): 0-070601-6.doi: 10.11889/j.0253-3219.2019.hjs.42.070601

• NUCLEAR ENERGY SCIENCE AND ENGINEERING •

Distribution of atmospheric multi-forms tritium in the vicinity of Qinshan nuclear power plants

Qingsong XU^1,²,Lailai QIN²(),Zhenghai XIA³,Zhongqin DAI⁴,Wei LIU²,Taijun PAN¹()

1. School of Material Science and Engineering, Jiangsu Key Laboratory of Material Surface Technology, Changzhou University, Changzhou 213164, China
2. Shanghai Institute of Applied Physics, Chinese Academy of Sciences, Shanghai 201800, China
3. China National Nuclear Corporation, Nuclear Power Operations Management Co. , Ltd, Haiyan 314300, China
4. Wuhan University, Wuhan 430072, China

Received:2019-04-08 Revised:2019-05-20 Online:2019-07-10 Published:2019-07-16
Contact: Lailai QIN,Taijun PAN E-mail:qinlailai@sinap.ac.cn;tjpan@cczu.edu.cn
About author:XU Qingsong, male, born in 1991, graduated from Jinling Institute of Technology in 2015, master student, focusing on distribution of atmospheric multi-forms tritium concentration

1	Aeschbach-Hertig W , Hofer M , Schmid M , et al . The physical structure and dynamics of a deep, meromictic crater lake (Lac Pavin, France)[J]. Hydrobiologia, 2002, 487(1): 111-136. DOI: 10.1023/a:1022942226198 . doi: 10.1023/a:1022942226198
2	Okai T , Momoshima N , Takashima Y . Variation of atmospheric tritium concentrations in three different chemical forms in Fukuoka, Japan[J]. Journal of Radioanalytical & Nuclear Chemistry, 1999, 239(3): 527-531. DOI: 10.1007/BF02349063 . doi: 10.1007/BF02349063
3	Atwood David A . Radionuclides in the environment[M]. United Kingdom: John Wiley & Sons Ltd, 2010: 47-65. DOI: 10.1007/978-3-319-22171-7 . doi: 10.1007/978-3-319-22171-7
4	Ansari M A , Mohokar H V , Deodhar A , et al . Distribution of environmental tritium in rivers, groundwater, mine water and precipitation in Goa, India[J]. Journal of Environmental Radioactivity, 2018, 189: 120-126. DOI: 10.1016/j.jenvrad.2018.04.004 . doi: 10.1016/j.jenvrad.2018.04.004
5	Uda T , Sugiyama T , Tanaka M , et al . Developments of gaseous water, hydrogen and methane sampling system for environmental tritium monitoring[J]. Fusion Engineering and Design, 2006, 81(8-14): 1385-1390. DOI: 10.1016/j.fusengdes.2005.08.077 . doi: 10.1016/j.fusengdes.2005.08.077
6	Liu C C , Chao J , Lin C C . Tritium release from nuclear power plants in Taiwan[J]. Health Physics, 2003, 84(3): 361-367. DOI: 10.1097/00004032-200303000-00009 . doi: 10.1097/00004032-200303000-00009
7	Yang Y H , Kang D W , Lee G B . Evaluation of ¹⁴C release characteristics in Korean standard pressurized water reactor[J]. Nuclear Engineering & Design, 2010, 240(10): 3611-3615. DOI: 10.1016/j.nucengdes.2010.03.034 . doi: 10.1016/j.nucengdes.2010.03.034
8	Å Magnusson . Carbon-14 produced by nuclear power reactors – generation and characterization of gaseous, liquid and solid waste[D]. Sweden: Lund University, 2007.
9	Shaver M W, Lanning D D . Secondary startup neutron sources as a source of tritium in a pressurized water reactor (PWR) reactor coolant system (RCS)[R]. United States of America: Pacific Northwest National Laboratory, 2010.
10	Kirchmann R , Meuricebourdon M , Fagniart E , et al . Purification resins in reactor circuits as source for organic tritium[J]. Radiation Protection Dosimetry, 1986, 16(1): 45-48. DOI: 10.1093/oxfordjournals.rpd.a079711 . doi: 10.1093/oxfordjournals.rpd.a079711
11	Eckerman K , Harrison J , Menzel H G , et al . ICRP publication 119: compendium of dose coefficients based on ICRP publication 60[J]. Annals of the ICRP, 2012, 41(supp_S1): 1-130. DOI: 10.1016/j.icrp.2012.06.038 . doi: 10.1016/j.icrp.2012.06.038
12	Boyer C V L , Fromm M , Losset Y , et al . Tritium in plants: a review of current knowledge[J]. Environmental & Experimental Botany, 2009, 67(1): 34-51. DOI: 10.1016/j.envexpbot.2009.06.008 . doi: 10.1016/j.envexpbot.2009.06.008
13	Akata N , Kakiuchi H , Shima N , et al . Tritium concentrations in the atmospheric environment at Rokkasho, Japan before the final testing of the spent nuclear fuel reprocessing plant[J]. Journal of Environmental Radioactivity, 2011, 102(9): 837-842. DOI: 10.1016/j.jenvrad.2011.05.005 . doi: 10.1016/j.jenvrad.2011.05.005
14	Tanaka M , Uda T . Variation of atmospheric tritium concentration in three chemical forms at Toki, Japan: 2004-12[J]. Radiation Protection Dosimetry, 2015, 167(1-3): 187-191. DOI: 10.1093/rpd/ncv241 . doi: 10.1093/rpd/ncv241
15	秦来来 . 核设施周围大气中多形态氚的测量[J]. 核技术, 2018, 41(10): 100604. DOI: 10.11889/j.0253-3219.2018.hjs.41.100604 . doi: 10.11889/j.0253-3219.2018.hjs.41.100604
	QIN Lailai . Measurement of atmospheric tritium in different chemical forms in the vicinity of nuclear facilities[J]. Nuclear Techniques, 2018, 41(10): 100604. DOI: 10.11889/j.0253-3219.2018.hjs.41.100604 . doi: 10.11889/j.0253-3219.2018.hjs.41.100604
16	秦来来 . 核设施周围大气中多形态氚监测方法研究[D]. 上海: 中国科学院上海应用物理研究所, 2018.
	Qin Lailai . Methodology study on measurement of multiform atmospheric tritium in the vicinity of nuclear facilities[D]. Shanghai: Shanghai Institute of Applied Physics, Chinese Academy of Sciences, 2018.
17	Jung-Seok C , Guebuem K . Dispersion and removal characteristics of tritium originated from nuclear power plants in the atmosphere[J]. Journal of Environmental Radioactivity, 2018, 192: 524-531. DOI: 10.1016/j.jenvrad.2018.08.007 . doi: 10.1016/j.jenvrad.2018.08.007
18	Deng K , Wang L , Xia Z H , et al . Tritium concentrations in precipitation in Shanghai[J]. Nuclear Science and Techniques, 2018, 29(5): 63. DOI: 10.1007/s41365-018-0412-2 . doi: 10.1007/s41365-018-0412-2
19	Du L , Zhang Q , Xia Z H , et al . Occurrence of HTO and NE-OBT in soil in the vicinity of the Qinshan Nuclear Power Plant[J]. Nuclear Science and Techniques, 2016, 27(4): 77. DOI: 10.1007/s41365-016-0087-5 . doi: 10.1007/s41365-016-0087-5
20	Inoue Y , Kahn B , Carter M W . Performances of an atmospheric tritium sampler and its application[J]. Japan Health Physics, 2010, 18(2): 119-127. DOI: 10.5453/jhps.18.119 . doi: 10.5453/jhps.18.119
21	Okai T , Momoshima N , Takashima Y . Variation of atmospheric tritium concentrations in three different chemical forms in Fukuoka, Japan[J]. Journal of Radioanalytical & Nuclear Chemistry, 1999, 239(3): 527-531. DOI: 10.1007/BF02349063 . doi: 10.1007/BF02349063
22	Okai T , Takashima Y . Analytical method for atmospheric tritium with a portable tritium sampling system[J]. Journal of Radioanalytical & Nuclear Chemistry, 1989, 130(2): 399-407. DOI: 10.1007/BF02041358 . doi: 10.1007/BF02041358
23	陈竹舟, 王守恕, 张茂栓, 等 . 秦山核电厂厂址地区的大气扩散实验研究[J]. 辐射防护, 1989, 9(6): 401-424. DOI: 10.1007/BF02005959 . doi: 10.1007/BF02005959
	CHEN Zhuzhou , WANG Shoushu , ZHANG Maoshuan , et al . Atmospheric diffusion experimental study in Qinshan Nuclear Power Plants base[J]. Radiation Protection, 1989, 9(6): 401-424. DOI: 10.1007/BF02005959 . doi: 10.1007/BF02005959
24	Xiang Y , Kan W , Zhang Y , et al . Radioactivity monitoring in environmental water and air around QNPP[J]. Nuclear Science and Techniques, 2007, 18(5): 316-320.
25	ICRP . ICRP Pulication 30: limits for intakes of radionuclides by workers[M]. London: Sega Publication Ltd, 1979.
26	Jung-Seok C , Guebuem K . Dispersion and removal characteristics of tritium originated from nuclear power plants in the atmosphere[J]. Journal of Environmental Radioactivity, 2018, 192: 524-531. DOI: 10.1016/j.jenvrad.2018.08.007 . doi: 10.1016/j.jenvrad.2018.08.007
27	杨海兰, 温雪莲, 张彩虹, 等 . 大亚湾核电站1997~2004年的氚监测及内照剂量评价[C]. 全国职业照射个人剂量监测与评价学术研讨会论文汇编, 2004.
	YANG Hailan , WEN Xuelian , ZHANG Caihong , et al . Tritium monitoring and dose evaluation of internal radiation in Daya Bay Nuclear Power Station from 1997 to 2004[C]. Papers of the Symposium on Monitoring and Evaluation of Personal Dose of Occupational Exposure, 2004.
28	Koarashi J , Mikami S , Akiyama K , et al . Determination of chemical forms of ³H released to the atmosphere from the Tokai reprocessing plant[J]. Journal of Radioanalytical & Nuclear Chemistry, 2004, 262(3): 569-572. DOI: 10.1007/s10967-005-0477-3 . doi: 10.1007/s10967-005-0477-3
29	Fujita H , Kokubun Y , Koarashi J . Environmental tritium in the vicinity of Tokai reprocessing plant[J]. Journal of Nuclear Science & Technology, 2007, 44(11): 1474-1480. DOI: 10.1080/18811248.2007.9711395 . doi: 10.1080/18811248.2007.9711395
30	Connan O , Hébert D , Solier L , et al . Atmospheric tritium concentrations under influence of AREVA NC La Hague reprocessing plant (France) and background levels[J]. Journal of Environmental Radioactivity, 2017, 177: 184-193. DOI: 10.1016/j.jenvrad.2017.06.015 . doi: 10.1016/j.jenvrad.2017.06.015

[1]	HOU Cheng, YU Tao, XIE Jinsen, ZENG Wenjie, CHEN Zhenping, XIE Qin, LIU Zijing, ZHAO Pengcheng, HE Lihua. The effects of the shape function and weighting function on the kinetics of the ADS sub-critical reactor [J]. Nuclear Techniques, 2018, 41(9): 90602-090602.
[2]	HE Linfeng, TANG Fangdong, ZHAO Chao. A method to determine the response coefficient of environmental gamma spectrometer to airborne radionuclide concentration [J]. Nuclear Techniques, 2018, 41(8): 80401-080401.
[3]	ZHENG Yunfei, LI Lanjun, KUANG Zhonghua, WANG Xiaohui, YANG Qian, SANG Ziru, REN Ning, WU San, FU Xin, YANG Yongfeng. Effects of light guide thickness on the performance of PET detectors consisting of high-resolution LYSO and SiPM array [J]. Nuclear Techniques, 2018, 41(4): 40403-040403.
[4]	XIA Sanqiang, LIU Liye, CAO Qinjian, HU Ling, LI Gang, ZHENG Minggui, HU Zhibin. On-site monitoring the activity concentration of nuclide ⁵⁸Co in coolant during PWR oxygenation shutdown [J]. Nuclear Techniques, 2018, 41(12): 120603-120603.
[5]	QIN Lailai, XIA Zhenghai, GU Shaozhong, MA Yuhua, DENG Ke, LIU Jiayu, MA Zhaowei, ZHANG Qin, YANG Guo, WEI Fei, WU Shengwei, BAO Guangliang, LIU Guimin, LIU Wei. Measurement of atmospheric tritium in different chemical forms in the vicinity of nuclear facilities [J]. Nuclear Techniques, 2018, 41(10): 100604-100604.
[6]	LI Qi, WANG Shilian, FAN Yuanqing, ZHAO Yungang, ZHANG Xinjun, JIA Huaimao, LIU Shujiang, CHANG Yinzhong. Accurate measurement of ¹³¹Xe^m activity concentration by internal gas proportional counting system [J]. Nuclear Techniques, 2018, 41(1): 10403-010403.
[7]	CHEN Li, GU Min, ZENG Guoqiang, GE Liangquan, YANG Kun, XIAO Ming. Radon daughter subtraction algorithm for artificial radioactive aerosol based on neural network [J]. Nuclear Techniques, 2017, 40(9): 90402-090402.
[8]	DENG Mingjun, WANG Yong, XUE Chaofan, TAI Renzhong. Theoretical simulation and experimental study on double white light interference system [J]. Nuclear Techniques, 2017, 40(8): 80103-080103.
[9]	QUAN Zheng, WANG Zhigang, WANG Junjing, DONG Yongwei, BAI Yonglin, BAO Tianwei, LIU Xin, LI Ran, LI Yong, WU Bobing, WANG Ruijie, WANG Le, WANG Bo, YAN Peng, XU Ming, ZHANG Li. Application of ICCD to the readout system for 3D imaging calorimeter [J]. Nuclear Techniques, 2017, 40(5): 50401-050401.
[10]	HE Houjun, XU Xiaohui, LU Yongkai, ZOU Jianxin, WANG Qiang, GUAN Xingcai, ZHAO Jiangtao, WANG Tieshan. Study of deposition behavior of deuterium in palladium using D-D nuclear reaction [J]. Nuclear Techniques, 2017, 40(2): 20201-020201.
[11]	ZHANG Hengquan, LI Jia, ZHU Qingjun, WU Yuxiao, NIE Xingchen. A solution to “long history” in the method of GVR based on weight window [J]. Nuclear Techniques, 2017, 40(12): 120602-120602.
[12]	LUAN Guangyuan, WANG Qi, BAO Jie, RUAN Xichao, REN Jie, JING Hantao, ZHANG Kai, HUANG Hanxiong. Physical design of fast fission chamber for neutron spectrum and flux measurement at the CSNS backstreaming white neutron source [J]. Nuclear Techniques, 2017, 40(11): 110501-110501.
[13]	QIN Lianjing, LI Meili, JIANG Lan, SONG Haiqing. Radioactivity characteristics of atmospheric aerosol samples in Guangzhou [J]. Nuclear Techniques, 2016, 39(9): 90501-090501.
[14]	ZHANG Yuxuan, YE Yongjun, XIAO Detao, JIANG Junting, DING Dexin, ZHONG Yongming, XIE Chao. Concentration distribution rules and characteristics of radon and its progeny in blind roadway with exhaust ventilation [J]. Nuclear Techniques, 2016, 39(5): 50202-050202.
[15]	WANG Tingting, WANG Liang, MO Zhaohong, ZHAO Deshan, XIONG Zhonghua. Theoretical simulation and experimental research of the light output function of liquid scintillator EJ339A [J]. Nuclear Techniques, 2016, 39(5): 50403-050403.

Distribution of atmospheric multi-forms tritium in the vicinity of Qinshan nuclear power plants

RichHTML

PDF (PC)

Like

Knowledge

Abstract

Cite this article

share this article

Figures/Tables 4

References 30

Related Articles 15

Metrics

Comments

Recommended 10